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1-105 of 105
- 1964–19681hTV-G5.1 (74)TV EpisodeSolo and Kuryakin investigate a plot in Ghupat, a nation in the Himalayas.
- 1964–19681hTV-G8.0 (100)TV EpisodeSolo and Kuryakin, aboard the Adriatic Express from Vienna to Venice, are seeking a Thrush chemical that can end the reproductive process in life forms. We meet Madame Nemirovitch, who claims to be the founder of Thrush.
- 1964–19681hTV-G7.4 (119)TV EpisodeA mysterious U.S. industrialist, Mr. Alexander, steals a new type of nerve gas from the U.S. Army. He leaves behind a small tablet with the number eight on it. Solo and Kuryakin investigate, with the help of Alexander's ex-wife Tracey, who seeks Alexander to sign her final divorce papers. The trio finds Alexander's parents working like slaves at a Greece rock quarry with the number five painted all around. After freeing the parents (and avoiding Alexander's thugs), they travel to a temple where they are captured by Alexander. It turns out Alexander plans to take over an Asian nation, breaking each of the Ten Commandments along the way.
- 1964–19681hTV-G7.3 (113)TV EpisodeSolo, Kuryakin and Tracey escape Alexander's death trap. The scene shifts to Washington and Virginia. Alexander breaks commandment No. 7 by seducing a prince's wife. He is planning on breaking No. 6 (Thou Shall Not Kill) and when that is done, his plot will be complete. Solo is menaced by a muscular thug while Kuryakin is endangered by employees of Alexander's farm in Virginia.
- Solo (Robert Vaughn) faces Thrush agents, a girl (Jeannine Reilly), her shotgun-toting father (Gil Lamb) and a preacher (Dub Taylor), as he and Kuryakin (David McCallum) search for exploding apples.
- Thrush, at a base in the Middle East, is developing a "vaporizer," which dissolves almost any object. Kuryakin tries to enlist the assistance of a tribe of Arabs to help. Solo, meanwhile, convinces a soon-to-be retired Thrushman that he'll live longer if he switches sides.
- Count Zark, a Thrush agent, operates out of Transylvania and has developed a worldwide menace involving bats. Meanwhile, UNCLE is checking out a young woman who seems capable of reading the minds of others. Solo and Kuryakin discover how both events are related.
- 1964–19681hTV-G7.4 (91)TV EpisodeThrush wipes out UNCLE's Geneva station with a strain of small, almost invisible, killer bees. The criminal organization next wants to use the bees on UNCLE's New York headquarters.
- A relative of Waverly's is being threatened if he doesn't sell shares in a company at a fraction of their value. Kuryakin is assigned to the affair, where his knowledge of gypsies proves useful. Solo, recuperating from a knee injury, provides limited assistance.
- Thrush poisons Waverly, with plans to subject him to a procedure that affects the brain. The criminal organization has already experimented on others, turning a shipping magnate and a diplomat into failures.
- 1964–19681hTV-G7.5 (95)TV EpisodeA scientist has developed a machine that reverses the aging process. UNCLE races Thrush for the device. An aging British politician and his manipulative wife will be key players in the outcome.
- 1964–19681hTV-G7.3 (88)TV EpisodeA British politician's career is suddenly rejuvenated after he's been exposed to a device that reverses the aging process. But he's also a prisoner. He needs additional treatments and the machine is now under the control of Thrush and the politician's manipulative wife.
- 1964–19681hTV-G7.2 (71)TV EpisodeThrush kidnaps the wife of a U.S. presidential candidate and substitutes a double.
- Alexander Waverly is scheduled to receive an honorary degree at his alma mater, Blair University. UNCLE is on guard to protect Waverly against an assassination attempt by Thrush.
- 1964–19681hTV-G7.7 (95)TV EpisodeThe search for a volcano-activating device takes Napoleon Solo (Robert Vaughn) and Illya Kuryakin (David McCallum) to Japan, where they must find Thrush's Far East headquarters.
- 1964–19681hTV-G7.9 (100)TV EpisodeThrush is operating a school for boys which really is training young assassins. The school's next target is an UNCLE gathering of top officials.
- 1964–19681hTV-G6.1 (71)TV EpisodeUNCLE and Thrush are seeking a Thrush code book in Algiers.
- 1964–19681hTV-G7.6 (87)TV EpisodeThrush, led by the nervous Louis Strago and his assassin secretary Miss Diketon, has embarked on an ambitious project. The organization has recruited a Nazi scientist who once theorized by changing the Gulf Stream, you could make Iceland into a lush, green country and make Europe into a frozen wasteland. Thrush is prepared to make the scientist's dream a reality. By the end of Part I, Napoleon Solo faces a forced marriage to a relative of retired gangsters while Illya Kuryakin is being tortured by Miss Diketon.
- 1964–19681hTV-G7.8 (82)TV EpisodeNapoleon Solo sets off for a Thrush island, from where the criminal organization will fire nuclear missiles to alter the path of the Gulf Stream. During the course of events, Solo enters into an uneasy alliance with retired gangsters; Miss Diketon betrays Thrush leader Louis Strago; and Illya Kuryakin nearly drowns.
- Solo and Kuryakin are told to escort a captured Thrush official, Egon Stryker, to Washington. Meantime, Waverly transports a man the agents are told is a double for Stryker. A Thrush team keeps trying to whisk Stryker away.
- U.N.C.L.E. and Thrush race to find a Nazi scientist, who worked for Adolf Hitler, after an SS officer assigned to guard the scientist turns up dead. The scientist, who now teaches under the name Professor Amadeus, has Hitler in suspended animation. He needs a person with the same blood type of Hitler's; the Nazi leader will need a completely new blood supply to come out of suspended animation. Amadeus discovers that Solo is the right blood type...
- 1964–19681hTV-G7.2 (95)TV EpisodeSolo and Kuryakin lock horns with Colonel Hubris, a Thrush operative. They also run into trouble with the local police.
- Karmak, given up for dead by Napoleon Solo and Illya Kuryakin, kidnaps Kuryakin to extract his revenge on Solo. Solo must find Kuryakin, who is somewhere in a 10-block area of condemned buildings, before 6 a.m. or else the Russian UNCLE agent will die.
- 1964–19681hTV-G6.7 (73)TV EpisodeThrush hopes to use a "suspended animation" device, invented by Dr. A.C. Nillson, against UNCLE.
- The son of a Thrush scientist is one of the most brilliant minds ever. UNCLE seeks to prevent the boy from ever working for Thrush.