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- Stories spotlight Marvel comic book characters Captain America, The Incredible Hulk, Iron Man, The Mighty Thor and The Sub-Mariner.
- The patriotic sole recipient of a revolutionary body enhancement project battles evil as the star spangled defender of America.
- The adventures of a nuclear scientist cursed with the tendency to turning into a huge green brute under stress.
- An inventive munitions industrialist fights the forces of evil using a revolutionary suit of power armor.
- The contemporary adventures of the Norse god of thunder and lightning.
- The prince of the sunken city of Atlantis protects his home from all enemies both above and below the surface of the sea.
- A mouse claiming to be centuries old helps tell tales of great historical figures and events.
- Animated short shows a young couple, Jack and Penny, learning to use an Investment Company to make their savings grow to meet their financial goals. Produced for the National Association of Investment Companies.
- 1967–197015mTV-Y76.5 (190)TV EpisodeOut in the countryside, Peter escapes an accident with the help of his Spider-Man disguise, but discovers a cave, with Dr.Octopus in charge of some power machines due to rule the World. Doc Ock captures Spidey, then Miss Brant who happened to be in the area. The villain is keeping both prisoners as witnesses for his demonstration of power...
- 1967–197015mTV-Y76.4 (138)TV EpisodeSpider-Man faces Electro, a man capable to shoot lightning rods with his hand and traveling on electric lines to go to his next heist.
- After framing Spider-Man, Mysterio offers to kill the superhero for J. Jonah Jameson for a fee.
- 1967–197015mTV-Y76.5 (115)TV EpisodeSpider-Man fights the Vulture who is controlling a massive flock of birds. In the second segment, the Daily Bugle publisher hunts Spider-Man with a remote-controlled robot.
- 1967–197015mTV-Y76.7 (94)TV EpisodeThe Rhino sets a gold standard for his crime spree - by creating a statue of himself. Then, a mastermind uses a cow-boy and a thug to find blueprints to destroy New York. It's up to Spider-Man to foil and neutralize their evil plan.
- 1967–197015mTV-Y76.2 (109)TV EpisodeThe Green Goblin tries to make a pact with J.Jonah Jameson in order to catch Spider-Man. However, Spidey must beware of his foe's witching powers.
- Dr Noah Boddy releases Electro, the Green Goblin and the Vulture to confront Spider-Man in a series of showdowns. Then, a Chameleon-like criminal eludes police and Spider-Man alike.
- 1967–197015mTV-Y77.0 (95)TV EpisodeTrying to foil a mystery keeping the demolition of a playhouse, Spider-Man meets Blackwell the Magician who, behind his mischievous tricks, has a message to say to him...
- 1967–197015mTV-Y75.8 (89)TV EpisodeSpider-Man is back in Florida, where he must find the secret behind an old Spanish Fort, guarded by some would-be Conquistadors.
- 1967–197015mTV-Y76.2 (93)TV EpisodeAn exotic African idol is used to hypnotize Jameson into embezzling for a villain. A mysterious hooded figure is using robotic store mannequins to commit robberies.
- 1967–197015mTV-Y76.3 (96)TV EpisodeA series of heists are made by mythical creatures, ruled by a woman who holds a library. Spider-Man must put a stop to this before it goes too far...
- A bad case of the common cold complicates Spider-Man's efforts to stop The Rhino from stealing the components of a secret weapon.
- 1967–197015mTV-Y76.8 (93)TV EpisodeDoc Ock steals a device in order to rule the world. Spider-Man must do something to keep this evil mastermind to achieve his dreadful threat.
- 1967–197015mTV-Y76.8 (111)TV EpisodeThe Scorpion, a super-human creation designed to vanquish Spider-Man, has a lethal sting in his tail and he's ready to sting J. Jonah Jameson. The Sandman heists the priceless Goliath Diamond and Spider-Man is the fall guy for the crime.
- 1967–197015mTV-Y76.3 (93)TV EpisodeA fakir is giving a hard time to Spider-Man, especially that he is a clever magician who can send spells to animals to attack the hero.
- 1967–197015mTV-Y76.6 (90)TV EpisodeThe Flys, a.k.a. the Patterson Twins, are paroled and freed. However, Spider-Man does not believe this and for a reason: they are framing him for all the heists they've done. It's up to Spidey to catch them in their act.
- In order to do a final battle with Spider-Man, the Vulture abducts J.Jonah Jameson and puts him next to a revolving pendulum. It's up to Spidey to stop the Vulture, otherwise his other nemesis Jamieson ends up in two halves.
- 1967–197015mTV-Y76.6 (105)TV EpisodeEscaped from jail, Electro is trying to find, then trap Spiderman for revenge.
- 1967–197015mTV-Y76.5 (93)TV EpisodeSpider-Man must stop a magnetism wielding mad scientist. Spidey must rescue a foreign prime minister that only he knows is kidnapped by an imposter.
- 1967–197015mTV-Y76.7 (95)TV EpisodeSpider-Man must stop a couple of former clever circus acrobats, dressed in dark, specialized in robbing big bank safes...
- When a city bank mysteriously vanishes into the street, J. Jonah Jameson sends a reporter named Hammond to investigate, while sending Peter to visit a scientist who has recorded voices supposedly from the center of the earth. Peter visits the scientist, and when a recording is played for him, he discovers it is the men - or beasts - who made the bank disappear, and they are plotting another one. Realizing it is only a few minutes until the plot is carried out, Peter becomes Spidey & heads for the bank. Sure enough, the bank disappears into the earth! Spidey follows it down & finds a strange kingdom of creatures - the Mole-Men. When the leader announces a plan to subjugate the people who were in the building when it was taken, Spidey moves into action & overpowers the Mole-Men, and both they & their hostages will be in for a surprise...
- Hoping to break up the love between Thor and Jane Foster, Odin heeds advice from Loki. Loki uses this opportunity to pit the Enchantress, the Executioner, and two powerful giants against Thor.
- Loki enhances the mental powers of Sandu, a carnival mystic. Sandu then uses his supernatural powers of levitation to battle Thor and to trap him beneath an entire building.
- When the Greek god Hercules arrives on Earth, he takes a fancy towards Thor's love Jane Foster. An enraged Thor fights it out with Hercules all over New York City.
- Thor's nemesis Loki forges an alliance with supervillains Mr Hyde and the Cobra. The trio kidnap Jane Foster to lure Thor into a booby-trap.
- When a race of underground lava men threaten the surface world with destruction, Thor gathers his Avenger teammates in an attempt to thwart the attack. The group is aided by an unlikely ally, their former team member, the Incredible Hulk.
- Loki lures a hunter into The Temple of Darkness, a hidden tomb where the hunter's spirit enters the body of the Indestructible Destroyer, an enchanted suit of armor forged by Odin.
- Escaped convict Crusher Creel is given power by Loki to absorb the properties of anything that he touches. As the Absorbing Man, Creel uses his fantastic strength to battle Thor.
- Scientist Paul Duval gains the power to turn himself (and whoever he touches) into living stone. As the Grey Gargoyle, he attacks Thor hoping to steal Thor's magic hammer, which he believes will help him gain immortality.
- Calvin Zabo, an employee fired by Donald Blake for stealing, vows revenge and uses a chemical formula to turn himself into the super powered Mr. Hyde.
- Zarrko, the Tomorrow Man, travels back in time to 1962 to steal a cobalt bomb that he plans on using to make himself ruler of the 23rd century. Thor follows him forward to 2262 in order to defeat him.
- After years of imprisonment in Asgard, Loki escapes to Earth to gain his revenge on his half-brother, Thor. Once there, Loki learns that Thor lives among humans as one of them, Dr. Donald Blake.
- Loki brings Jane Foster to Asgard and tries to convince Odin that it was Thor who brought her there. In order to prove which of his sons is lying, Odin sends both to Skornheim, where they must endure its deadly dangers.
- Tricked into signing a contract to become the ruler of the underworld, Hercules must rely upon Thor to champion his cause and help him to win his freedom.
- 19666.0 (37)TV EpisodeThe world's greatest expert on electricity devises a robot to destroy Iron Man.
- 19666.5 (45)TV EpisodeThe Mandarin attacks Tony Stark's house but Pepper and others suspect Iron Man may be to blame.
- While Tony Stark is busy with his new race car one of his scientists plots to destroy him.
- 1966TV-G5.9 (77)TV EpisodeA quick recap of how Steve Rodgers became Captain America/Captain America's main focus is on saboteurs as he keeps his identity secret by being an army private/Captain America learns that the Red Skull is behind the sabotage.
- 1966TV-G4.9 (55)TV EpisodeSurprised to learn that Captain America is still alive, Zemo plots an all out attack.
- 1966TV-G5.8 (50)TV EpisodeCaptain America leads the Avengers into Sin-Cong to answer a distress call, only to find it's a trap set by the nation's superhuman leader, the Commissar.
- Tony Stark is held prisoner by the Mandarin, whose latest minion is the giant android Ultimo.